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Free, publicly-accessible full text available January 4, 2025
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Zhang, Xue-Hao ; Mohanty, Soumya D. ; Zou, Xiao-Bo ; Liu, Yu-Xiao ( , Physical Review D)
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Qu, Shizhen ; Chaudhary Nagar, Garima ; Li, Wenkai ; Liu, Kun ; Zou, Xiao ; Hon Luen, Seck ; Dempsey, Dennis ; Hong, Kyung-Han ; Jie Wang, Qi ; Zhang, Ying ; et al ( , Optics Letters)
We experimentally demonstrate long-wavelength-infrared (LWIR) femtosecond filamentation in solids. Systematic investigations of supercontinuum (SC) generation and self-compression of the LWIR pulses assisted by laser filamentation are performed in bulk KrS-5 and ZnSe, pumped by
, 9 µm, 10 µJ pulses from an optical parametric chirped-pulse amplifier operating at 10 kHz of repetition rate. Multi-octave SC spectra are demonstrated in both materials. While forming stable single filament, 1.5 cycle LWIR pulses with 4.5 µJ output pulse energy are produced via soliton-like self-compression in a 5 mm thick KrS-5. The experimental results quantitatively agree well with the numerical simulation based on the unidirectional pulse propagation equation. This work shows the experimental feasibility of high-energy, near-single-cycle LWIR light bullet generation in solids.